Manipulating Electrocatalysis using Mosaic Catalysts

نویسندگان

چکیده

Understanding the mechanisms and developing strategies toward efficient electrocatalysis at gas–liquid–solid interfaces are important yet challenging. In past decades, researchers have devoted many efforts to improve catalyst activity by modulating electronic properties of catalysts in terms chemical components physical features. Herein, a mosaic catalyst, which is defined as with spatially isolated periodically distributed active areas, developed dramatically catalysts. Taking Pt an example, leads high catalytic performance, showing specific 11 times higher than that uniform films for hydrogen evolution reaction (HER), well current densities commercial Pt/C films. Such strategy found be general other (e.g., 2D PtS) reactions oxygen reaction). The improved performance attributed enhanced mass transferability local electric field strength, both determined occupation ratios work shines new light on manipulating from perspective spatial structures catalysts, guides design heterogeneous reactions.

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ژورنال

عنوان ژورنال: Small science

سال: 2021

ISSN: ['2688-4046']

DOI: https://doi.org/10.1002/smsc.202000059